Key Laboratory of Low-dimensional Quantum Structures and Quantum Control of Ministry of Education, College of Physics and Information Science, Hunan Normal University, Changsha 410081, China
† Corresponding author. E-mail: zhmzc1997@126.com
Project supported by the Science and Technology Plan of Hunan Province, China (Grant No. 2010FJ3148), the National Natural Science Foundation of China (Grant No. 11374096), and the Doctoral Science Foundation of Hunan Normal University, China.
1. IntroductionEntanglement, as a kind of quantum correlation,[1,2] is considered to be not only a vital concept in physics but also a prime resource for quantum information processing.[3,4] Therefore, a great deal of attention has been devoted to the experimental generation and manipulation of entangled systems and the theoretical study of the entanglement evolution.[5,6] In particular, since Yu and Eberly[7] discovered that the Markovian entanglement dynamics of two qubits exposed to local noisy environments may markedly differ from the single-qubit decoherence evolution, the analysis of entanglement decay and its relation with decoherence induced by an unavoidable interaction between a system and its environment has become an important topic. Many important progresses have been acquired in experimental and theoretical researches on entanglement dynamics in open quantum systems. The investigations show that environmental noises can not only be helpful to protect entanglement, but also can make entanglement sudden death (ESD), entanglement sudden birth (ESB), and entanglement swapped.[8–10]
However, entanglement is not the only type of quantum correlation useful for quantum information processing. Ollivier and Zurek introduced another concept of quantum correlation, termed discord,[11,12] which captures nonclassical correlations, including but not limited to entanglement, that is, separability of a density matrix describing a two-qubit system does not guarantee vanishing of discord. Discord has significant applications in deterministic quantum computation with one pure qubit (DQC1)[13] and estimation of quantum correlations in the Grover search algorithm.[14] On the other hand, discord has also been extensively used in studies of quantum phase transition[15,16] and to measure the quantum correlation between relatively accelerated observers.[17]
A realistic physical system always suffers from some unwanted interactions with its outside environments,[18] causing decoherence and destroying entanglement and discord. This interaction of a quantum system with its environment may be described using either a classical or a quantum mechanical picture of the environment. Understanding whether and in which conditions the two descriptions are equivalent is still a debated topic.[19–22] When the environment has many degrees of freedom and/or a structured noise spectrum, a classical description may be convenient and also more accurate. Several systems of interest belong to these categories and many efforts have been devoted to study situations where quantum systems are affected by the classical noise. Examples include the dynamics of quantum correlations[23–26] and the decoherence in solid state qubits.[27,28] But a quantum mechanical description of an open system is usually thought of as being a more general approach. In recent years, many methods and important progresses have been acquired in studying open systems using the quantum mechanical picture of the environment. For instance, Bellomo et al. studied the entanglement dynamics of two independent qubits in non-Markovian environments.[29,30] Xiao et al.[31] discussed the discord dynamics of two qubits in this model. In Refs. [30]–[33], the same model is adopted, in which the whole system can be divided into two parts and a formal solution for the evolution may be obtained by exactly solving the time-dependent Schrödinger equation in the subspace with one excitation.
In this paper, we apply the time-convolutionless (TCL) master-equation method to investigate discord and entanglement of two atoms immersed in two independent Lorentzian reservoirs, in which the two atoms and the two reservoirs are included as a whole system. We focus on the influences of temperatures, atomic initial states, and non-Markovian effect as well as detuning on discord and entanglement. Firstly, we find that the nonzero temperature can induce the entanglement sudden death and accelerate the decays of discord and entanglement. Secondly, the discord and entanglement have different robustness for the different initial states and their robustness may change under certain conditions. Thirdly, when both the non-Markovian effect and detuning are present simultaneously, due to the memory and feedback effect of the non-Markovian reservoirs, the discord and entanglement can be effectively protected even at the nonzero temperature by increasing the non-Markovian effect and the detuning.
The report is structured as follows. We present a physical model in Section 2. In Section 3, we introduce discord and entanglement of a two-qubit system. Results and a discussion are given in Section 4. We conclude the report briefly in Section 5.
2. Physical modelWe consider two two-level atoms, where each atom couples with a structured reservoir.[34] The Hamiltonian is (ħ = 1) H = H0 + αHI, where is the free Hamiltonian of the combined system, ω0 is the transition frequency of the atom, is the inversion operators describing the atom j (j = A or B), and bn,A(bm,B) are the creation and annihilation operators of the reservoir with the frequency ωn,A(ωm,B). The parameter α is a dimensionless expansion parameter. In the interaction picture, the Hamiltonian αHI reads
where
gn,j is the coupling constant between the atom and its reservoir,
and
are the upward and downward operators of the atom, respectively.
In the second-order approximation, the TCL master equation[18] of ρAB(t) has the form [HI(τ),ρAB(t)⊗ρE]]) with the environment state ρE. Here, we have supposed that ρ(t) = ρAB(t)⊗ρE and TrE([HI(t),ρAB(0)⊗ρE]) = 0, thus the TCL master equation may be written as
where
is the Liouville super-operator
[35] defined by
The correlation functions
kj(
t) and
fj(
t) are given by
and
where 〈
O〉
Ej ≡ Tr
Ej(
OρEj).
Assuming that the two reservoirs are identical and initially prepared in a thermal state with temperature T, the correlation functions reduce to
Here,
kB is the Boltzmann constant. For a sufficiently large environment, we can replace the sum over the discrete coupling constants with an integral over a continuous distribution of frequencies of the environmental modes, i.e.,
Let the spectral density have a Lorentzian form
where
δ is the detuning between
ω0 and the reservoir center frequency
ω. The parameter
λ defines the spectral width of the coupling, which is connected to the reservoir correlation time
τR by
τR=
λ−1 and the parameter
γ0 is related to the relaxation time scale
τS by
In the subsequent analysis, typically weak and strong coupling regimes can be distinguished. For a weak regime,
λ > 2
γ0 (i.e.,
τS > 2
τR), the dynamical behavior of the system is essentially a Markovian exponential decay controlled by
γ0. In the strong coupling regime,
λ < 2
γ0 (i.e.,
τS < 2
τR), the non-Markovian effects become relevant.
[36]Inserting Eq. (7) into Eq. (6), we obtain the correlation functions
3. Discord and entanglementFor any two-qubit system ρAB, its total correlation can be written as where S(ρ) = –Tr(ρ log2ρ) is the von Neumann entropy[2] of ρ. Its classical correlation is here the maximum represents the most information gained about subsystem A as a result of the perfect measurement {Πk} on subsystem B. The is the quantum conditional entropy of subsystem A: and are the probability and the state of subsystem A for measurement outcome k. Discord is defined as the difference between the total correlation and the classical correlation i.e.,
and is interpreted as a measurement of quantum correlations.
[11] For the X state, described by the following density matrix:
Discord can be calculated,
[37] analytically, as
where
with
λk being the eigenvalues of
ρAB and
h(
x) = –
xlog
2x–(1 –
x)log
2(1 –
x) is the binary entropy. Here,
D1 =
h(
τ), where
and
In addition to discord, another quantum correlation is entanglement, which can be calculated through entanglement of formation (EoF), as[38]
where
H(
x) = –
xlog
2x – (1 –
x)log
2(1 –
x),
is Wootter’s concurrence and
λi are the eigenvalues, organized in descending order, of the matrix
For the X state such as Eq. (
10), the concurrence of
ρAB is
[9]Discord is equal to entanglement for pure states, but their relation is complicated for the mixed states, that is, there are separable mixed states with nonzero discord.[39] In the following, our main concern will be the dynamic behaviors of discord and entanglement of two atoms in Lorentzian reservoirs at zero and finite temperatures.
4. Results and discussionIn the section, we discuss in detail the dynamic behaviors of discord (D) and entanglement (E) of two atoms in Lorentzian reservoirs. If the initial atomic states are
the atomic density matrix
ρAB(
t) can remain an X structure under the master equation Eq. (
2). Utilizing Eqs. (
11) and (
12), we can calculate the discord and entanglement of
ρAB(
t). In the following discussion, we first give the dynamic evolutions of discord and entanglement in the resonant case, then we analyze those in the non-resonant case.
4.1. Resonant caseWe assume that the two atoms couple resonantly to the Lorentzian reservoirs (i.e., δ = 0) and study the influence of the temperature, the non-Markovian effect, and the initial states on the discord and entanglement.
4.1.1. Case I: The Markovian regimeFigure 1 presents the dynamics of discord and entanglement for different initial states and different temperatures under λ = 5γ0 and δ = 0.
Figure 1(a) displays the dynamics of discord and entanglement for |ψ(0)〉 at T = 0. The results show that, both the discord and entanglement decay exponentially and vanish asymptotically, and their robustness can change at the critical time, which is expressed by tcri and γ0tcri = 0.32, namely, the discord reduces slightly faster than the entanglement when γ0t < 0.32 while the discord is more robust than the entanglement when γ0t > 0.32. Figure 1(b) gives the dynamics of discord and entanglement for |ϕ(0)〉 and T = 0. Comparing Fig. 1(a) with Fig. 1(b), we find that the discord for |ϕ(0)〉 is a little more robust than that for |ψ(0)〉, and likewise for the entanglement. Also γ0tcri = 0.6, namely, the tcri for |ϕ(0)〉 is bigger than that for |ψ(0)〉.
When kBT/ħω0 = 1, the dynamic behaviors of discord and entanglement for |ψ(0)〉 and |ϕ(0)〉 are respectively plotted in Figs. 1(c) and 1(d). In Fig. 1(c), there is γ0tcri = 0.22, and it is worth noting that the discord still reduces quickly and asymptotically to zero but the entanglement can vanish completely in a very short time, i.e., ESD, whose time is expressed by tESD and γ0tESD = 0.73. In Fig. 1(d), there are γ0tcri = 0.22 and γ0tESD = 0.78, so the entanglement behavior in Fig. 1(d) is very similar to that in Fig. 1(c) except that the entanglement decay in Fig. 1(d) is a little slower than that in Fig. 1(c), and likewise for the discord. Namely, the initial states hardly affect the discord and entanglement at nonzero temperature, which is markedly different from that in the zero temperature case.
Comparing Figs. 1(c) and 1(d) with Figs. 1(a) and 1(b) respectively, we can see that, nonzero temperature can accelerate the decays of the discord and entanglement and shorten tcri. More importantly, nonzero temperature can yet induce the ESD. The reason is that the thermal effect of the environment can enhance the atomic dissipation so that the discord and entanglement reduce more quickly and the discord is more robust against temperature than the entanglement.
Therefore, under the resonance and the Markovian regime, the discord for |ϕ(0)〉 is more robust than that for |ψ(0)〉, and likewise for the entanglement. Nonzero temperature can accelerate the decays of the discord and entanglement and induce the ESD.
4.1.2. Case II: The non-Markovian regimeFigure 2 depicts the evolutions of discord and entanglement versus γ0t for different initial states and different temperatures under λ = 0.1 γ0 and δ = 0.
Figure 2(a) shows that, for T = 0 and |ψ(0)〉, both the discord and entanglement decay exponentially and vanish asymptotically after a short time, and γ0tcri = 1.84. Figure 2(b) describes that, for T = 0 and |ϕ(0)〉, the discord and entanglement will also reduce asymptotically to zero and γ0tcri = 3.0. Comparing Fig. 2(b) with Fig. 2(a), we find that, the discord for |ϕ(0)〉 is also more robust than that for |ψ(0)〉, and likewise for the entanglement. Figures 2(c) and 2(d) respectively give the discord and entanglement for |ψ(0)〉 and |ϕ(0)〉 at kBT/ħω0 = 1. Figure 2(c) tells us that, γ0tcri = 1.2 and γ0tESD = 3.0. In Fig. 2(d), there are γ0tcri = 1.2 and γ0tESD = 3.1, so the entanglement behavior in Fig. 2(d) is very similar to that in Fig. 2(c) except that the decay of the entanglement in Fig. 2(d) is a little slower than that in Fig. 2(c), and likewise for the discord. Comparing Figs. 2(c) and 2(d) with Figs. 2(a) and 2(b) respectively, it can be observed that, nonzero temperature can also accelerate the decays of the discord and entanglement and induce the ESD.
Comparing Figs. 2(a)–2(d) with Figs. 1(a)–1(d) respectively, we know that, in the resonance, the non-Markovian effect can reduce the decay rates of the discord and entanglement and prolong tcri and tESD, but these influences are very small.
4.2. Non-resonant caseAbove, we have restricted our discussion to the resonant case, but the detuning case (i.e., δ ≠ γ0) would be more reasonable.
4.2.1. Case I: The Markovian regimeFigure 3 displays the dynamics of discord and entanglement for different initial states and different temperatures under λ = 5γ0 and δ = γ0. Comparing Fig. 3 with Fig. 1, we see that, the decay rates of discord in Figs. 3(a)–3(d) are approximately equal to those in Figs. 1(a)–1(d) respectively, and likewise for the entanglement. However, the tESD in Figs. 3(c) and 3(d) is a little bigger than that in Figs. 1(c) and 1(d), respectively. As a result, in the Markovian regime, the detuning hardly impacts on the discord and entanglement.
4.2.2. Case II: The non-Markovian regimeFigure 4 exhibits the influence of initial states and temperatures on the discord and entanglement when both the non-Markovian effect and the detuning are present simultaneously (i.e., λ = 0.1γ0 and δ = γ0).
Figure 4(a) gives the dynamic behaviors of discord and entanglement for |ψ(0)〉 at T = 0. In this case, due to the memory and feedback effect of reservoirs, both the discord and entanglement can oscillate damply then reduce asymptotically to zero over a long time (see the inset in Fig. 4(a)) and γ0tcri = 7.7. In a short time (γ0t ≤ 40), both the discord and entanglement are obviously protected. The relations of the discord and entanglement versus γ0t for |ϕ(0)〉 at T = 0 are plotted in Fig. 4(b). It is seen that, γ0tcri = 31, and both the discord and entanglement are also obviously protected. Comparing Figs. 4(b) and 4(a), it is very evident that the discord for |ϕ(0)〉 reduces much slower than that for |ψ(0)〉, and likewise for the entanglement.
In Figs. 4(c) and 4(d), we draw the dynamics of discord and entanglement for |ψ(0)〉 and |ϕ(0)〉 at kBT/ħω0 = 1. Figure 4(c) shows that, for |ψ(0)〉, there is γ0tcri = 1.2 and the discord and entanglement all oscillate damply then the discord decreases asymptotically to zero but the entanglement will be sudden death at γ0tESD = 33. In Fig. 4(d) (for |ϕ(0)〉), there are γ0tcri = 1.2 and γ0tESD = 34, that is, the discord behavior in Fig. 4(d) is very similar to that in Fig. 4(c), and likewise for the entanglement. Comparing Figs. 4(c) and 4(d) with Figs. 4(a) and 4(b) respectively, it can show that, nonzero temperature can accelerate the decays of discord and entanglement, enlarge the oscillating amplitudes of discord and entanglement and induce the ESD even if both the non-Markovian effect and detuning are present simultaneously.
Comparing Fig. 4 with Figs. 2 and 3, we find that they are essentially different. If there is only the non-Markovian effect or only the detuning, the discord and entanglement will monotonously and rapidly decline to zero. However, if the non-Markovian effect and the detuning are present simultaneously, the discord and entanglement will oscillate damply and their decay rates also evidently become smaller. The physical interpretation is that, when only λ < 2γ0 (the non-Markovian effect) or only δ ≠ 0 (the detuning), the quantum information can flow out from the atomic system but is hardly returned from the reservoirs so that the discord and entanglement monotonously and rapidly reduce, as shown in Figs. 2 and 3. However, when λ < 2γ0 and δ ≠ 0, due to the memory and feedback effect of the non-Markovian reservoir, the quantum information flowing to the reservoir will be partly returned to the atom so that the discord and entanglement oscillate damply and their decay rates become smaller, as shown in Fig. 4.
Figure 5 reveals the dynamics of discord and entanglement under λ = 0.1γ0 and δ = 4γ0. From Fig. 5(a), we see that, for |ψ(0)〉 and T = 0, the discord and entanglement can be effectively protected and the entanglement is more robust than the discord when γ0t ≤ 40 although they can reduce asymptotically to zero over a very long time (see the inset in Fig. 5(a)). Figure 5(b) shows that the discord for |ϕ(0)〉 is more robust than that for |ψ(0)〉, and likewise for the entanglement. Figure 5(c) states clearly that, the discord and entanglement can still be effectively protected at kBT/ħω0 = 1, but their decay rates and oscillating amplitudes are a little bigger than those at T = 0. The entanglement in Fig. 5(d) is similar to that in Fig. 5(c) expect that the decay rate in Fig. 5(d) is a little smaller than that in Fig. 5(c), and likewise for the discord.
Comparing Figs. 5(a)–5(d) with Fig. 4(a)–4(d) respectively, we know that, in the non-Markovian regime, increasing the detuning can prolong tcri and tESD (see the insets in Fig. 5), enlarge the oscillating frequency and reduce the decays of discord and entanglement. More importantly, even at nonzero temperature, the discord and entanglement can also be effectively protected by means of the big detuning. The physical explanation is that, in the non-Markovian regime, with δ increasing, the atom can more quickly exchange the quantum information with its reservoir so that the atomic decay becomes slower and the quantum information returned from the reservoir is more, hence the discord and entanglement can be more effectively protected.
Figure 6 exhibits the dynamics of discord and entanglement under λ = 0.01γ0 and δ = γ0. From Fig. 6(a), we see that, for |ψ(0)〉 and T = 0, the discord and entanglement can be effectively protected when γ0t ≤ 40 although the discord and entanglement yet reduce asymptotically to zero in a very long time (see the inset in Fig. 6(a)). Figure 6(b) reveals that, for |ϕ(0)〉 and T = 0, the discord for |ϕ(0)〉 is more robust than that for |ψ(0)〉, and likewise for the entanglement. Figure 6(c) tells us that, the discord and entanglement can also be effectively protected at kBT/ħω0 = 1, but their decay rates and oscillating amplitudes are a little larger than those at T = 0. The entanglement in Fig. 6(d) is very similar to that in Fig. 6(c) expect that the decay rate in Fig. 6(d) is a little smaller than that in Fig. 6(c), and likewise for the discord.
Comparing Figs. 6(a)–6(d) with Figs. 4(a)–4(d) respectively, we know that, under the detuning, increasing the non-Markovian effect can prolong tcri and tESD (see the insets in Fig. 6) and reduce the decays of discord and entanglement. More importantly, even at nonzero temperature, the discord and entanglement can also be effectively protected by means of the strong non-Markovian effect. The physical explanation is that, under the detuning, with λ decreasing, the memory and feecback effect of the non-Markovian reservoir can become strong so that the atomic decay becomes slower and the quantum information returned from the reservoir is more, hence the discord and entanglement can be more effectively protected.
5. ConclusionIn the present work, we have investigated the dynamics of discord and entanglement of two atoms in Lorentzian reservoirs at zero and nonzero temperatures by using the time-convolutionless master-equation method. We find that, the discord and entanglement markedly rely on the non-Markovian effect, the detuning, and the temperature as well as the atomic initial states. The entanglement is more robust than the discord when t < tcri while the discord is more robust than the entanglement when t > tcri, and the value of tcri relies on the initial states, the temperature, the detuning, and the non-Markovian effect. The discord for |ϕ(0)〉 is always more robust than that for |ψ(0)〉, specially, this difference is very evident at the zero temperature, and likewise for the entanglement. The nonzero temperature can accelerate the decays of discord and entanglement and induce the entanglement sudden death. More importantly, if there is only the detuning or only the non-Markovian effect, both the discord and entanglement will monotonously and rapidly decline to zero. However, if the non-Markovian effect and the detuning are present simultaneously, due to the memory and feedback of the non-Markovian reservoir, the discord and entanglement will oscillate damply and both of them can be effectively protected even at the nonzero temperature by increasing the detuning and the non-Markovian effect. These results will be useful in quantum computation and quantum information processing.
The current experimental technologies[40] show that our proposals have a certain feasibility. For example, a circular Rydberg atom with the two circular levels with principal quantum numbers 51 and 50 which are called |e〉 and |g〉 respectively, the |e〉 ⇔ |g〉 transition is at 51.1 GHz corresponding to the atomic decay rate γ0 = 33.3 Hz. Indeed, in the above discussion, the detuning δ = 2γ0 = 66.6 Hz is very small so that it could be realized by Stark-shifting the frequency with a static electric field. The typical Stark shift is about 200 kHz,[41] which is far more than 66.6 Hz. This shift is therefore large enough to effectively preserve the discord and entanglement. Moreover, in cavity QED experiments, ultrahigh finesse Fabry–Perot super-conducting resonant cavities with quality factors Q = 4.2 × 1010, corresponding to the spectral width λ = 7 Hz, have been realized.[42] These values correspond to λ/γ0 ≈ 0.2 which represents a good non-Markovian regime. Moreover, from Figs. 5 and 6, we may know that, the discord and entanglement can be effectively protected when γ0t ≤ 40 (meaning a corresponding time on the scale of seconds) and kBT/ħω0 = 1 (meaning the order of T ∼ 10−8 K), these conditions may be realized in the current experimental technologies.